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dc.contributor.author | De Bruijckere, J. | |
dc.contributor.author | Gehring, P. | |
dc.contributor.author | Palacios-Corella, M. | |
dc.contributor.author | Clemente León, Miguel | |
dc.contributor.author | Coronado Miralles, Eugenio | |
dc.contributor.author | Paaske, J. | |
dc.contributor.author | Hedegård, P. | |
dc.contributor.author | Van der Zant, H. S. J. | |
dc.date.accessioned | 2020-04-06T09:07:50Z | |
dc.date.available | 2020-04-06T09:07:50Z | |
dc.date.issued | 2019 | |
dc.identifier.citation | De Bruijckere, J. Gehring, P. Palacios-Corella, M. Clemente León, Miguel Coronado Miralles, Eugenio Paaske, J. Hedegård, P. Van der Zant, H.S.J. 2019 Ground-State Spin Blockade in a Single-Molecule Junction Physical Review Letters 122 197701-1 197701-5 | |
dc.identifier.uri | https://hdl.handle.net/10550/73778 | |
dc.description.abstract | It is known that the quantum mechanical ground state of a nanoscale junction has a significant impact on its electrical transport properties. This becomes particularly important in transistors consisting of a single molecule. Because of strong electron-electron interactions and the possibility of accessing ground states with high spins, these systems are eligible hosts of a current-blockade phenomenon called a ground-state spin blockade. This effect arises from the inability of a charge carrier to account for the spin difference required to enter the junction, as that process would violate the spin selection rules. Here, we present a direct experimental demonstration of a ground-state spin blockade in a high-spin single-molecule transistor. The measured transport characteristics of this device exhibit a complete suppression of resonant transport due to a ground-state spin difference of 3/2 between subsequent charge states. Strikingly, the blockade can be reversibly lifted by driving the system through a magnetic ground-state transition in one charge state, using the tunability offered by both magnetic and electric fields. | |
dc.language.iso | eng | |
dc.relation.ispartof | Physical Review Letters, 2019, vol. 122, p. 197701-1-197701-5 | |
dc.subject | Partícules (Física nuclear) | |
dc.subject | Quàntums, Teoria dels | |
dc.title | Ground-State Spin Blockade in a Single-Molecule Junction | |
dc.type | journal article | es_ES |
dc.date.updated | 2020-04-06T09:07:50Z | |
dc.identifier.doi | 10.1103/PhysRevLett.122.197701 | |
dc.identifier.idgrec | 134323 | |
dc.rights.accessRights | open access | es_ES |