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Towards peptide-based tunable multistate memristive materials

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Towards peptide-based tunable multistate memristive materials

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dc.contributor.author Cardona Serra, Salvador
dc.contributor.author Rosaleny Peralvo, Lorena Estefanía
dc.contributor.author Giménez-Santamarina, Silvia
dc.contributor.author Martínez-Gil, Luis
dc.contributor.author Gaita Ariño, Alejandro
dc.date.accessioned 2021-05-07T08:14:01Z
dc.date.available 2021-05-08T04:45:05Z
dc.date.issued 2020 es_ES
dc.identifier.citation Salvador Cardona-Serra, Lorena E. Rosaleny, Silvia Giménez-Santamarina, Luis Martínez-Gil, Alejandro Gaita-Ariño, Phys. Chem. Chem. Phys., 2021, 23, 1802-1810 es_ES
dc.identifier.uri https://hdl.handle.net/10550/79239
dc.description.abstract Development of new memristive hardware is a technological requirement towards widespread neuromorphic computing. Molecular spintronics seems to be a fertile field for the design and preparation of this hardware. Within molecular spintronics, recent results on metallopeptides demonstrating the interaction between paramagnetic ions and the chirality induced spin selectivity effect hold particular promise for developing fast (ns–μs) operation times. [R. Torres-Cavanillas et al., J. Am. Chem. Soc., 2020, DOI: 10.1021/jacs.0c07531]. Among the challenges in the field, a major highlight is the difficulty in modelling the spin dynamics in these complex systems, but at the same time the use of inexpensive methods has already allowed progress in that direction. Finally, we discuss the unique potential of biomolecules for the design of multistate memristors with a controlled- and indeed, programmable-nanostructure, allowing going beyond anything that is conceivable by employing conventional coordination chemistry. es_ES
dc.description.abstract Development of new memristive hardware is a technological requirement towards widespread neuromorphic computing. Molecular spintronics seems to be a fertile field for the design and preparation of this hardware. Within molecular spintronics, recent results on metallopeptides demonstrating the interaction between paramagnetic ions and the chirality induced spin selectivity effect hold particular promise for developing fast (ns–μs) operation times. [R. Torres-Cavanillas et al., J. Am. Chem. Soc., 2020, DOI: 10.1021/jacs.0c07531]. Among the challenges in the field, a major highlight is the difficulty in modelling the spin dynamics in these complex systems, but at the same time the use of inexpensive methods has already allowed progress in that direction. Finally, we discuss the unique potential of biomolecules for the design of multistate memristors with a controlled- and indeed, programmable-nanostructure, allowing going beyond anything that is conceivable by employing conventional coordination chemistry. en_US
dc.description.sponsorship European Research Council es_ES
dc.description.sponsorship European Cooperation in Science & Tecnology es_ES
dc.description.sponsorship Ministerio de Ciencia, Innovación y Universidades es_ES
dc.description.sponsorship Generalitat Valenciana-Prometeo Program of Excellence es_ES
dc.description.sponsorship es_ES
dc.description.sponsorship Universitat de València
dc.language.iso es es_ES
dc.title Towards peptide-based tunable multistate memristive materials es_ES
dc.type journal article es_ES
dc.subject.unesco UNESCO::QUÍMICA es_ES
dc.identifier.doi 10.1039/D0CP05236A es_ES
dc.identifier.idgrec 142855 es_ES
dc.accrualmethod - es_ES
dc.embargo.terms 0 days es_ES
dc.relation.projectID PRECOMP14-202646
dc.relation.projectID CEX2019-000919-M
dc.relation.projectID CTQ2017-8952
dc.relation.projectID COST-MOLSPIN-CA15128
dc.relation.projectID ERC-CoG DECRESIM 647301

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