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Multivariate sodalite zeolitic imidazolate frameworks: a direct solvent-free synthesis

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Multivariate sodalite zeolitic imidazolate frameworks: a direct solvent-free synthesis

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dc.contributor.author	López Cabrelles, Javier
dc.contributor.author	Miguel‐Casañ, Eugenia
dc.contributor.author	Esteve-Rochina, María
dc.contributor.author	Andres-Garcia, Eduardo
dc.contributor.author	Vitórica-Yrezábal, Iñigo J.
dc.contributor.author	Calbo Roig, Joaquín
dc.contributor.author	Mínguez Espallargas, Guillermo
dc.date.accessioned	2022-02-23T14:27:23Z
dc.date.available	2022-02-23T14:27:23Z
dc.date.issued	2022
dc.identifier.citation	López Cabrelles, Javier Miguel&#8208Casañ, Eugenia Esteve-Rochina, María Andres-Garcia, Eduardo Vitórica-Yrezábal, Iñigo J. Calbo Roig, Joaquín Mínguez Espallargas, Guillermo 2022 Multivariate sodalite zeolitic imidazolate frameworks: a direct solvent-free synthesis Chemical Science 13 3 842 847
dc.identifier.uri	https://hdl.handle.net/10550/81699
dc.description.abstract	Different mixed-ligand Zeolitic Imidazolate Frameworks (ZIFs) with sodalite topology, i.e. isoreticular to ZIF-8, unachievable by conventional synthetic routes, have been prepared using a solvent-free methodology. In particular, the versatility of this method is demonstrated with three different metal centres (Zn, Co and Fe) and binary combinations of three different ligands (2-methylimidazole, 2-ethylimidazole and 2-methylbenzimidazole). One combination of ligands, 2-ethylimidazole and 2-methylbenzimidazole, results in the formation of SOD frameworks for the three metal centres despite this topology not being obtained for the individual ligands. Theoretical calculations confirm that this topology is the lowest in energy upon ligand mixing.
dc.language.iso	eng
dc.relation.ispartof	Chemical Science, 2022, vol. 13, num. 3, p. 842-847
dc.subject	Materials
dc.subject	Compostos orgànics Síntesi
dc.title	Multivariate sodalite zeolitic imidazolate frameworks: a direct solvent-free synthesis
dc.type	journal article	es_ES
dc.date.updated	2022-02-23T14:27:23Z
dc.identifier.doi	10.1039/D1SC04779E
dc.identifier.idgrec	150444
dc.rights.accessRights	open access	es_ES