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Strong optical nonlinearities in gallium and indium selenides related to inter-valence-band transitions induced by light pulses

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Strong optical nonlinearities in gallium and indium selenides related to inter-valence-band transitions induced by light pulses

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dc.contributor.author Segura García del Río, Alfredo
dc.contributor.author Bouvier, Jaqueline
dc.contributor.author Andrés, Miguel V.
dc.contributor.author Manjón Herrera, Francisco Javier
dc.contributor.author Muñoz Sanjosé, Vicente
dc.date.accessioned 2022-03-11T18:12:17Z
dc.date.available 2022-03-11T18:12:17Z
dc.date.issued 1997
dc.identifier.citation Segura García del Río, Alfredo Bouvier, Jaqueline Andrés, Miguel V. Manjón Herrera, Francisco Javier Muñoz Sanjosé, Vicente 1997 Strong optical nonlinearities in gallium and indium selenides related to inter-valence-band transitions induced by light pulses Physical Review B 56 7 4075 4084
dc.identifier.uri https://hdl.handle.net/10550/81927
dc.description.abstract A nonlinear optical effect is shown to occur in gallium and indium selenides at photon energies of the order of 1.5 eV. It corresponds to transitions from a lower-energy valence band to the uppermost one when a nonequilibrium degenerate hole gas is created in the latter by a laser pulse. This inter-valence-band transition is allowed by crystal symmetry. Its oscillator strength is estimated through the f-sum rule and turns out to be about two orders of magnitude higher than that of the fundamental transition. The intensity of this effect is stronger when the pump pulse photon energy is close to that of the inter-valence-band transition; a condition that can be fulfilled only in indium selenide. The transient behavior of the sample transmittance is shown to be controlled by the balance between absorption and stimulated emission, which depends on the hole quasi-Fermi level and the gap renormalization due to Coulomb interaction in the electron-hole gas generated by the pump.
dc.language.iso eng
dc.relation.ispartof Physical Review B, 1997, vol. 56, num. 7, p. 4075-4084
dc.subject Òptica
dc.title Strong optical nonlinearities in gallium and indium selenides related to inter-valence-band transitions induced by light pulses
dc.type journal article es_ES
dc.date.updated 2022-03-11T18:12:17Z
dc.identifier.doi 10.1103/PhysRevB.56.4075
dc.identifier.idgrec 081079
dc.rights.accessRights open access es_ES

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