We perform the first magnetohydrodynamic simulations in full general relativity of self-consistent rotating neutron stars (NSs) with ultrastrong mixed poloidal and toroidal magnetic fields. The initial uniformly rotating NS models are computed assuming perfect conductivity, stationarity, and axisymmetry. Although the specific geometry of the mixed field configuration can delay or accelerate the development of various instabilities known from analytic perturbative studies, all our models finally succumb to them. Differential rotation is developed spontaneously in the cores of our magnetars which, after sufficient time, is converted back to uniform rotation. The rapidly rotating magnetars show a significant amount of ejecta, which can be responsible for transient kilonova signatures. However no highly collimated, helical magnetic fields or incipient jets, which are necessary for gamma-ray bursts, arise at the poles of these magnetars by the time our simulations are terminated.