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Efficient and Thermally Stable Wide Bandgap Perovskite Solar Cells by Dual-Source Vacuum Deposition

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Efficient and Thermally Stable Wide Bandgap Perovskite Solar Cells by Dual-Source Vacuum Deposition

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dc.contributor.author Bolink, Henk
dc.contributor.author Susic, Isidora
dc.contributor.author Gil Escrig, Lidón
dc.contributor.author Doğan, İlker
dc.contributor.author Zardetto, Valerio
dc.contributor.author Najafi, Mehrdad
dc.contributor.author Zhang, Dong
dc.contributor.author Veenstra, Sjoerd
dc.contributor.author Sedani, Salar
dc.contributor.author Arikan, Bulent
dc.contributor.author Yerci, Selçuk
dc.contributor.author Sessolo, Michele
dc.date.accessioned 2023-09-11T10:53:45Z
dc.date.available 2023-09-11T10:53:45Z
dc.date.issued 2023
dc.identifier.citation Bolink, Henk Susic, Isidora Gil Escrig, Lidón Do&#287an, &#304lker Zardetto, Valerio Najafi, Mehrdad Zhang, Dong Veenstra, Sjoerd Sedani, Salar Arikan, Bulent Yerci, Selçuk Sessolo, Michele 2023 Efficient and Thermally Stable Wide Bandgap Perovskite Solar Cells by Dual-Source Vacuum Deposition Advanced Functional Materials 33 2214357 1 11
dc.identifier.uri https://hdl.handle.net/10550/89186
dc.description.abstract Wide bandgap perovskites are being widely studied in view of their potential applications in tandem devices and other semitransparent photovoltaics. Vacuum deposition of perovskite thin films is advantageous as it allows the fabrication of multilayer devices, fine control over thickness and purity, and it can be upscaled to meet production needs. However, the vacuum processing of multicomponent perovskites (typically used to achieve wide bandgaps) is not straightforward, because one needs to simultaneously control several thermal sources during the deposition. Here a simplified dual-source vacuum deposition method to obtain wide bandgap perovskite films is shown. The solar cells obtained with these materials have similar or even larger efficiency as those including multiple A-cations, but are much more thermally stable, up to 3500 h at 85 °C for a perovskite with a bandgap of 1.64 eV. With optimized thickness, record efficiency of >19% and semitransparent devices with stabilized power output in excess of 17% are achieved.
dc.language.iso eng
dc.relation.ispartof Advanced Functional Materials, 2023, vol. 33, num. 2214357, p. 1-11
dc.subject Materials
dc.subject Química
dc.title Efficient and Thermally Stable Wide Bandgap Perovskite Solar Cells by Dual-Source Vacuum Deposition
dc.type journal article
dc.date.updated 2023-09-11T10:53:45Z
dc.identifier.doi 10.1002/adfm.202214357
dc.identifier.idgrec 160980
dc.rights.accessRights open access

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