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Vacuum deposited wide bandgap perovskite solar cells

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Vacuum deposited wide bandgap perovskite solar cells

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dc.contributor.advisor Bolink, Henk
dc.contributor.advisor Sessolo, Michele
dc.contributor.author Susic, Isidora
dc.contributor.other Facultat de Química es_ES
dc.date.accessioned 2023-10-27T08:13:13Z
dc.date.available 2023-10-28T04:45:07Z
dc.date.issued 2023 es_ES
dc.date.submitted 27-10-2023 es_ES
dc.identifier.uri https://hdl.handle.net/10550/90728
dc.description.abstract Wide bandgap perovskite solar cells have demonstrated great potential for multi-junction solar cells applications. This thesis aims to develop efficient wide bandgap perovskite solar cells fabricated using scalable techniques, in particular using vacuum deposition methods. The focus is on improving the properties of wide bandgap perovskite films and incorporating them into high-performing solar cells. The time-consuming nature of laboratory-scale thermal evaporation deposition is addressed by developing a combinatorial vacuum deposition approach. This enables the rapid development of novel perovskite compositions by producing over 100 solar cells with different compositions in a single deposition run. Furthermore, a strategy to increase the complexity of the formulation of vacuum-deposited lead halide perovskites films is introduced, and efficient and thermally stable CsMAFAGA quadruple-cation perovskite solar cells were prepared. Finally, the stabilization of the CsPbI3 black perovskite phase via vacuum deposition is investigated. CsPbI3 perovskite films were successfully obtained at room temperature by incorporating a larger cation, dimethylammonium. Moreover, fully vacuum processed solar cells are fabricated in both the p-i-n and n-i-p configurations, incorporating these CsPbI3 perovskite films. es_ES
dc.format.extent 162 p. es_ES
dc.language.iso en es_ES
dc.subject perovskite solar cells es_ES
dc.subject vacuum deposition es_ES
dc.title Vacuum deposited wide bandgap perovskite solar cells es_ES
dc.type doctoral thesis es_ES
dc.subject.unesco UNESCO::QUÍMICA es_ES
dc.embargo.terms 0 days es_ES
dc.rights.accessRights open access es_ES

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